Changing pulse-shape basis for molecular learning control

David Cardoza, Florian Langhojer, Carlos Trallero-Herrero, Oliver L A Monti Masel, Thomas Weinacht

Research output: Contribution to journalArticle

28 Citations (Scopus)

Abstract

The results of a molecular fragmentation learning control experiment were analyzed. An amplified Ti:sapphire laser system capable of producing 30-fs pulses with an energy of ∼1 mJ at a repetition rate of 1 kHz was used for the experiment. The experiments involved fragmentation of trifluoroacetone. A time-of flight mass spectrometer (TOFM) was used to evaluate the pulse shapes. The time domain basis was found to be natural for cases where periodic dynamics play a key role in selective fragmentation.

Original languageEnglish (US)
Article number053406
JournalPhysical Review A
Volume70
Issue number5 B
DOIs
StatePublished - Nov 2004

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learning
fragmentation
pulses
mass spectrometers
repetition
sapphire
lasers
energy

ASJC Scopus subject areas

  • Atomic and Molecular Physics, and Optics
  • Physics and Astronomy(all)

Cite this

Cardoza, D., Langhojer, F., Trallero-Herrero, C., Monti Masel, O. L. A., & Weinacht, T. (2004). Changing pulse-shape basis for molecular learning control. Physical Review A, 70(5 B), [053406]. https://doi.org/10.1103/PhysRevA.70.053406

Changing pulse-shape basis for molecular learning control. / Cardoza, David; Langhojer, Florian; Trallero-Herrero, Carlos; Monti Masel, Oliver L A; Weinacht, Thomas.

In: Physical Review A, Vol. 70, No. 5 B, 053406, 11.2004.

Research output: Contribution to journalArticle

Cardoza, D, Langhojer, F, Trallero-Herrero, C, Monti Masel, OLA & Weinacht, T 2004, 'Changing pulse-shape basis for molecular learning control', Physical Review A, vol. 70, no. 5 B, 053406. https://doi.org/10.1103/PhysRevA.70.053406
Cardoza, David ; Langhojer, Florian ; Trallero-Herrero, Carlos ; Monti Masel, Oliver L A ; Weinacht, Thomas. / Changing pulse-shape basis for molecular learning control. In: Physical Review A. 2004 ; Vol. 70, No. 5 B.
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