Direct observation of rotational energy transfer in ammonia by time-resolved infrared-microwave double resonance

J. M. Levy, J. H.S. Wang, S. G. Kukolich, J. I. Steinfeld

Research output: Contribution to journalArticlepeer-review

22 Scopus citations

Abstract

An N2O laser is used to pump the ground vibrational state (8,7) inversion doublet of 14NH3 while simultaneously monitoring other ground state doublets. Time-resolved rotational energy transfer signals are observed in accordance with known selection values. Absolute rates of rotational energy transfer processes are estimated.

Original languageEnglish (US)
Pages (from-to)598-602
Number of pages5
JournalChemical Physics Letters
Volume21
Issue number3
DOIs
StatePublished - Sep 1 1973
Externally publishedYes

ASJC Scopus subject areas

  • Physics and Astronomy(all)
  • Physical and Theoretical Chemistry

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