Electron correlation in artificial atoms

Thomas M. Henderson, Keith Runge, Rodney J. Bartlett

Research output: Contribution to journalArticle

26 Scopus citations

Abstract

Electron correlation is essential to the accurate description of molecular systems. Here, parabolic quantum dots (often referred to as artificial atoms) are treated with the coupled cluster formalism of quantum chemistry to introduce correlation. Electron correlation is shown to account for between 1% and 9% of the total energy of quantum dots with from two to eight electrons and has a significant qualitative effect on the addition spectra. We employ a scaling relationship, confirmed by our calculations, which allows the treatment of quantum dots without specific reference to material properties.

Original languageEnglish (US)
Pages (from-to)138-142
Number of pages5
JournalChemical Physics Letters
Volume337
Issue number1-3
DOIs
StatePublished - Mar 30 2001
Externally publishedYes

ASJC Scopus subject areas

  • Physics and Astronomy(all)
  • Physical and Theoretical Chemistry

Fingerprint Dive into the research topics of 'Electron correlation in artificial atoms'. Together they form a unique fingerprint.

  • Cite this