Abstract
Nonlinear absorption spectra of quantum confined CdSe microcrystallites in glass are measured in a femtosecond pump-probe experiment at low temperatures. Simultaneous bleaching of the transitions, and an induced absorption at higher energy are observed. Spectral hole burning is observed as the pump is tuned through the transition. The system is modelled as spherical crystallites with one or two electron-hole pairs interacting through the Coulomb potential. A numerical matix diagonalization method predicts results essentially similar to the experiment and attributes them to state filling of the one-pair states, and generation of two-pair states.
| Original language | English (US) |
|---|---|
| Title of host publication | Proceedings of SPIE - The International Society for Optical Engineering |
| Editors | Nasser Peygambarian |
| Publisher | Publ by Int Soc for Optical Engineering |
| Pages | 98-104 |
| Number of pages | 7 |
| Volume | 1216 |
| ISBN (Print) | 0819402575 |
| State | Published - 1990 |
| Event | Nonlinear Optical Materials and Devices for Photonic Switching - Los Angeles, CA, USA Duration: Jan 16 1990 → Jan 17 1990 |
Other
| Other | Nonlinear Optical Materials and Devices for Photonic Switching |
|---|---|
| City | Los Angeles, CA, USA |
| Period | 1/16/90 → 1/17/90 |
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ASJC Scopus subject areas
- Electrical and Electronic Engineering
- Condensed Matter Physics
Cite this
Femtosecond hole-burning and nonlinear dynamics of quantum confined semiconductor-doped glasses. / Fluegel, B.; Koch, Stephan W; Peyghambarian, Nasser N; Hulin, D.; Migus, A.; Joffre, M.; Antonetti, A.
Proceedings of SPIE - The International Society for Optical Engineering. ed. / Nasser Peygambarian. Vol. 1216 Publ by Int Soc for Optical Engineering, 1990. p. 98-104.Research output: Chapter in Book/Report/Conference proceeding › Conference contribution
}
TY - GEN
T1 - Femtosecond hole-burning and nonlinear dynamics of quantum confined semiconductor-doped glasses
AU - Fluegel, B.
AU - Koch, Stephan W
AU - Peyghambarian, Nasser N
AU - Hulin, D.
AU - Migus, A.
AU - Joffre, M.
AU - Antonetti, A.
PY - 1990
Y1 - 1990
N2 - Nonlinear absorption spectra of quantum confined CdSe microcrystallites in glass are measured in a femtosecond pump-probe experiment at low temperatures. Simultaneous bleaching of the transitions, and an induced absorption at higher energy are observed. Spectral hole burning is observed as the pump is tuned through the transition. The system is modelled as spherical crystallites with one or two electron-hole pairs interacting through the Coulomb potential. A numerical matix diagonalization method predicts results essentially similar to the experiment and attributes them to state filling of the one-pair states, and generation of two-pair states.
AB - Nonlinear absorption spectra of quantum confined CdSe microcrystallites in glass are measured in a femtosecond pump-probe experiment at low temperatures. Simultaneous bleaching of the transitions, and an induced absorption at higher energy are observed. Spectral hole burning is observed as the pump is tuned through the transition. The system is modelled as spherical crystallites with one or two electron-hole pairs interacting through the Coulomb potential. A numerical matix diagonalization method predicts results essentially similar to the experiment and attributes them to state filling of the one-pair states, and generation of two-pair states.
UR - http://www.scopus.com/inward/record.url?scp=0025636968&partnerID=8YFLogxK
UR - http://www.scopus.com/inward/citedby.url?scp=0025636968&partnerID=8YFLogxK
M3 - Conference contribution
SN - 0819402575
VL - 1216
SP - 98
EP - 104
BT - Proceedings of SPIE - The International Society for Optical Engineering
A2 - Peygambarian, Nasser
PB - Publ by Int Soc for Optical Engineering
ER -