We demonstrate the creation and measurement of vibrational wavepackets in small polyatomic molecules using nonresonant impulsive excitation. Modeling reveals features due to vibrational dephasing and rephrasing, rotational dephasing, and dissociation.
|Original language||English (US)|
|Number of pages||3|
|Journal||Springer Series in Chemical Physics|
|State||Published - May 17 2003|
ASJC Scopus subject areas
- Physical and Theoretical Chemistry