Techno-economic Assessment for Integrating Biosorption into Rare Earth Recovery Process

Hongyue Jin, Dan M. Park, Mayank Gupta, Aaron W. Brewer, Lewis Ho, Suzanne L. Singer, William L. Bourcier, Sam Woods, David W. Reed, Laura N. Lammers, John W. Sutherland, Yongqin Jiao

Research output: Contribution to journalArticle

8 Scopus citations

Abstract

The current uncertainty in the global supply of rare earth elements (REEs) necessitates the development of novel extraction technologies that utilize a variety of REE source materials. Herein, we examined the techno-economic performance of integrating a biosorption approach into a large-scale process for producing salable total rare earth oxides (TREOs) from various feedstocks. An airlift bioreactor is proposed to carry out a biosorption process mediated by bioengineered rare earth-adsorbing bacteria. Techno-economic assessments were compared for three distinctive categories of REE feedstocks requiring different pre-processing steps. Key parameters identified that affect profitability include REE concentration, composition of the feedstock, and costs of feedstock pretreatment and waste management. Among the 11 specific feedstocks investigated, coal ash from the Appalachian Basin was projected to be the most profitable, largely due to its high-value REE content. Its cost breakdown includes pre-processing (leaching primarily, 77.1%), biosorption (19.4%), and oxalic acid precipitation and TREO roasting (3.5%). Surprisingly, biosorption from the high-grade Bull Hill REE ore is less profitable due to high material cost and low production revenue. Overall, our results confirmed that the application of biosorption to low-grade feedstocks for REE recovery is economically viable.

Original languageEnglish (US)
Pages (from-to)10148-10155
Number of pages8
JournalACS Sustainable Chemistry and Engineering
Volume5
Issue number11
DOIs
StatePublished - Nov 6 2017
Externally publishedYes

Keywords

  • Airlift bioreactor
  • Low-grade feedstock
  • Mineral recovery
  • Mining
  • TEA

ASJC Scopus subject areas

  • Chemistry(all)
  • Environmental Chemistry
  • Chemical Engineering(all)
  • Renewable Energy, Sustainability and the Environment

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  • Cite this

    Jin, H., Park, D. M., Gupta, M., Brewer, A. W., Ho, L., Singer, S. L., Bourcier, W. L., Woods, S., Reed, D. W., Lammers, L. N., Sutherland, J. W., & Jiao, Y. (2017). Techno-economic Assessment for Integrating Biosorption into Rare Earth Recovery Process. ACS Sustainable Chemistry and Engineering, 5(11), 10148-10155. https://doi.org/10.1021/acssuschemeng.7b02147